Finch co-wrote and directed an award-winning short film, The Day (1960) and announced plans to direct a feature but it did not eventuate. He won his third BAFTA for Best Actor for No Love for Johnnie (1961), although like Oscar Wilde, the film lost money. He was originally chosen to play Julius Caesar in Cleopatra (1963) and filmed scenes in London, but when the film was postponed he withdrew; the role was recast with Rex Harrison.
During his war service Finch was given leave to act in radio, theatre and film. He appeared in a number of propaganda shorts, including Another Threshold (1942), These Stars Are Mine (1943), While There is Still Time (1943) and South West Pacific (1943), the latter for Ken G. Hall. He also appeared in two of the few Australian feature films made during the war, The Rats of Tobruk (1944) and the less distinguished Red Sky at Morning (1944).
In 1954, the Australian journalist and author George Johnston wrote a well-researched series of biographical articles on Finch, his life, and his work, which appeared in the Sydney Sun-Herald on four consecutive Sundays, which were certainly the first detailed account of Finch's life to be published. Finch later provided the inspiration for the character Archie Calverton in Johnston's novel, Clean Straw for Nothing.
Finch was married three times. In 1943, he married Romanian-born French ballerina Tamara Tchinarova; they worked together on a number of films. They had a daughter, Anita, born in 1950. They divorced in 1959, after she discovered his affair with actress Vivien Leigh in California. He then married South African-born actress Yolande Turner (née Yolande Eileen Turnbull); they had two children together, Samantha and Charles Peter. During their marriage, Finch had an affair with the singer Shirley Bassey. Bassey had a daughter, also named Samantha, born in 1963; Bassey's husband at the time, the openly gay film producer Kenneth Hume, believed that Finch was her biological father. Finch and Turner divorced in 1965. In 1972 Finch married Mavis "Eletha" Barrett, who was known as Eletha Finch. They had a daughter together, Diana.
Finch's next three films saw him support notable female stars: Sophia Loren in Judith (1966), Melina Mercouri in 10:30 P.M. Summer (1966) and Julie Christie in Far from the Madding Crowd (1967). He was reunited with Aldrich for The Legend of Lylah Clare (1968). The Red Tent (1970) was an expensive international adventure film, with Finch as Umberto Nobile.
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He had a small role as an Australian prisoner of war in The Wooden Horse (1950), the third most popular film at the British box office in 1950. His performance as a Pole in Daphne Laureola led to his casting as a Polish soldier in The Miniver Story, the sequel to the wartime morale boosting film Mrs. Miniver; unlike its predecessor, it was poorly received critically.